Transition from nonsequential to sequential double ionization in many-electron systems

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dc.contributor.author Pullen, Michael G.
dc.contributor.author Wolter, Benjamin
dc.contributor.author Wang, Xu
dc.contributor.author Tong, Xiao-Min
dc.contributor.author Sclafani, Michele
dc.contributor.author Baudisch, Matthias
dc.contributor.author Pires, Hugo
dc.contributor.author Schröter, Claus Dieter
dc.contributor.author Ullrich, Joachim
dc.contributor.author Pfeifer, Thomas
dc.contributor.author Moshammer, Robert
dc.contributor.author Eberly, J. H.
dc.contributor.author Biegert, Jens
dc.date.accessioned 2019-04-18T13:51:22Z
dc.date.available 2019-04-18T13:51:22Z
dc.date.issued 2017-09-05
dc.identifier.uri http://hdl.handle.net/2097/39579
dc.description Citation: Pullen, M. G., Wolter, B., Wang, X., Tong, X.-M., Sclafani, M., Baudisch, M., … Biegert, J. (2017). Transition from nonsequential to sequential double ionization in many-electron systems. Physical Review A, 96(3), 033401. https://doi.org/10.1103/PhysRevA.96.033401
dc.description.abstract Understanding strong-field double ionization of many-electron systems is an important fundamental problem with potential implications for molecular imaging within this regime. Using mid-IR radiation, we unambiguously identify the transition from nonsequential (e, 2e) to sequential double ionization in Xe at an intensity below 1014W/cm2. Ionization from excited orbitals is found to be decisive at low intensities, but we demonstrate that such mechanisms are unimportant in the sequential regime. We utilize these facts to successfully image a molecular dication using laser-induced electron diffraction. This methodology can be used to study molecular dynamics on unprecedented few-femtosecond time scales.
dc.language.iso en_US
dc.relation.uri 10.1103/PhysRevA.96.033401
dc.rights ©2017 American Physical Society
dc.rights.uri https://journals.aps.org/authors/transfer-of-copyright-agreement
dc.rights.uri https://rightsstatements.org/page/InC/1.0/?language=en
dc.subject Electron & positron scattering
dc.subject Electron correlation calculations for atoms & ions
dc.subject Multiphoton or tunneling ionization & excitation
dc.subject Ultrafast phenomena
dc.title Transition from nonsequential to sequential double ionization in many-electron systems
dc.type Text
dc.date.published 2017
dc.citation.doi https://doi.org/10.1103/PhysRevA.96.033401
dc.citation.issn 1476-4688
dc.citation.issue 3
dc.citation.jtitle Physical Review A
dc.citation.spage 33401
dc.citation.volume 96
dc.citation Pullen, M. G., Wolter, B., Wang, X., Tong, X.-M., Sclafani, M., Baudisch, M., … Biegert, J. (2017). Transition from nonsequential to sequential double ionization in many-electron systems. Physical Review A, 96(3), 033401. https://doi.org/10.1103/PhysRevA.96.033401
dc.description.version Article: Version of Record (VoR)


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