Gearba, M. A.Camp, H. A.Trachy, M. L.Veshapidze, G.Shah, M. H.Jang, H. U.DePaola, B. D.2023-12-072023-12-072007-07-17https://hdl.handle.net/2097/43715The temporal evolution of populations has been directly measured for a three-level ladder system undergoing coherent excitation by stimulated Raman adiabatic passage (STIRAP). The measurement technique makes use of charge transfer as diagnostic. The method is model independent and has a temporal resolution of a few nanoseconds. The temporal evolution is measured for several values of the delay between the pump and Stokes laser pulses that are part of the STIRAP excitation scheme. The corresponding quantum Liouville equations are solved and the results of the calculations are compared with experiment.© American Physical Society (APS). This Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s).http://rightsstatements.org/vocab/InC/1.0/https://web.archive.org/web/20181120135245/https://journals.aps.org/copyrightFAQ.htmlText