Liao, QingThumm, Uwe P. E.2014-06-202014-06-202014-03-25http://hdl.handle.net/2097/17873We analyze the dependence of attosecond streaked photoelectron spectra and photoemission time delays from valence band (VB) and 2p core-level (CL) states of a single-crystalline Mg(0001) thin film on the (i) modeling of the substrate electronic structure, (ii) electron mean free path (MFP), (iii) screening of the near-infrared (NIR) streaking laser field, and (iv) chirp of the attosecond extreme ultraviolet (XUV) pulse. Our quantum-mechanical numerical simulations predict streaked photoemission spectra that depend sensitively on the XUV chirp and weakly on the screening of the streaking laser field by the substrate. They furthermore show that streaking time delays for VB emission are relatively insensitive to the modeling of the initial quantum states, electron MFP, and NIR skin depth of the Mg substrate, in contrast to the stronger dependence of streaking time delays for 2p CL emission on these factors.en-USThis Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s).Attosecond extreme ultraviolet (XUV) pulseStreaking traceStreaked photoemission spectraStreaking time delaysArticle (publisher version)