Tracing the photodissociation probability of H2+ in intense fields using chirped laser pulses

dc.citation.doi10.1103/PhysRevA.81.023401
dc.citation.issn1050-2947
dc.citation.issue2
dc.citation.jtitlePhysical Review A
dc.citation.volume81
dc.contributor.authorPrabhudesai, Vaibhav S.
dc.contributor.authorLev, Uri
dc.contributor.authorNatan, Adi
dc.contributor.authorBruner, Barry D.
dc.contributor.authorDiner, Adi
dc.contributor.authorHeber, Oded
dc.contributor.authorStrasser, Daniel
dc.contributor.authorSchwalm, D.
dc.contributor.authorBen-Itzhak, Itzik
dc.contributor.authorHua, J. J.
dc.contributor.authorEsry, B. D.
dc.contributor.authorSilberberg, Yaron
dc.contributor.authorZajfman, Daniel
dc.date.accessioned2023-12-07T18:23:45Z
dc.date.available2023-12-07T18:23:45Z
dc.date.issued2010-02-03
dc.date.published2010-02-03
dc.description.abstractThe temporal evolution of the dissociation probabilities for various vibrational levels of H2+ is observed in terms of shifts in the kinetic energy release dissociation spectra, induced by linearly chirped intense laser pulses. In contrast to previous observations, in which no dependence on the chirp sign was observed, the energy spectrum reported here shows peak shifts, up for negative chirp and down for positive chirp. For some vibrational levels, dissociation takes place early on in the pulse; hence, care must be taken while interpreting the effect of pulse duration in photodissociation studies. This interpretation is supported by numerical solutions of the time-dependent Schrödinger equation.
dc.identifier.urihttps://hdl.handle.net/2097/43829
dc.relation.urihttps://link.aps.org/doi/10.1103/PhysRevA.81.023401
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dc.titleTracing the photodissociation probability of H2+ in intense fields using chirped laser pulses
dc.typeText

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