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Coulomb-explosion imaging of concurrent ${\mathbf{CH}}_{2}\mathbf{BrI}$ photodissociation dynamics

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dc.citationBurt, M., Boll, R., Lee, J. W. L., Amini, K., Köckert, H., Vallance, C., … Rolles, D. (2017). Coulomb-explosion imaging of concurrent ${\mathbf{CH}}_{2}\mathbf{BrI}$ photodissociation dynamics. Physical Review A, 96(4), 043415. https://doi.org/10.1103/PhysRevA.96.043415
dc.citation.doi10.1103/PhysRevA.96.043415
dc.citation.issn1476-4689
dc.citation.issue4
dc.citation.jtitlePhysical Review A
dc.citation.spage43415
dc.citation.volume96
dc.contributor.authorBurt, Michael
dc.contributor.authorBoll, Rebecca
dc.contributor.authorLee, Jason W. L.
dc.contributor.authorAmini, Kasra
dc.contributor.authorKöckert, Hansjochen
dc.contributor.authorVallance, Claire
dc.contributor.authorGentleman, Alexander S.
dc.contributor.authorMackenzie, Stuart R.
dc.contributor.authorBari, Sadia
dc.contributor.authorBomme, Cédric
dc.contributor.authorDüsterer, Stefan
dc.contributor.authorErk, Benjamin
dc.contributor.authorManschwetus, Bastian
dc.contributor.authorMüller, Erland
dc.contributor.authorRompotis, Dimitrios
dc.contributor.authorSavelyev, Evgeny
dc.contributor.authorSchirmel, Nora
dc.contributor.authorTechert, Simone
dc.contributor.authorTreusch, Rolf
dc.contributor.authorKüpper, Jochen
dc.contributor.authorTrippel, Sebastian
dc.contributor.authorWiese, Joss
dc.contributor.authorStapelfeldt, Henrik
dc.contributor.authorde Miranda, Barbara Cunha
dc.contributor.authorGuillemin, Renaud
dc.contributor.authorIsmail, Iyas
dc.contributor.authorJournel, Loïc
dc.contributor.authorMarchenko, Tatiana
dc.contributor.authorPalaudoux, Jérôme
dc.contributor.authorPenent, Francis
dc.contributor.authorPiancastelli, Maria Novella
dc.contributor.authorSimon, Marc
dc.contributor.authorTravnikova, Oksana
dc.contributor.authorBrausse, Felix
dc.contributor.authorGoldsztejn, Gildas
dc.contributor.authorRouzée, Arnaud
dc.contributor.authorGéléoc, Marie
dc.contributor.authorGeneaux, Romain
dc.contributor.authorRuchon, Thierry
dc.contributor.authorUnderwood, Jonathan
dc.contributor.authorHolland, David M. P.
dc.contributor.authorMereshchenko, Andrey S.
dc.contributor.authorOlshin, Pavel K.
dc.contributor.authorJohnsson, Per
dc.contributor.authorMaclot, Sylvain
dc.contributor.authorLahl, Jan
dc.contributor.authorRudenko, Artem
dc.contributor.authorZiaee, Farzaneh
dc.contributor.authorBrouard, Mark
dc.contributor.authorRolles, Daniel
dc.date.accessioned2019-04-18T13:51:22Z
dc.date.available2019-04-18T13:51:22Z
dc.date.issued2017-10-17
dc.date.published2017
dc.descriptionCitation: Burt, M., Boll, R., Lee, J. W. L., Amini, K., Köckert, H., Vallance, C., … Rolles, D. (2017). Coulomb-explosion imaging of concurrent ${\mathbf{CH}}_{2}\mathbf{BrI}$ photodissociation dynamics. Physical Review A, 96(4), 043415. https://doi.org/10.1103/PhysRevA.96.043415
dc.description.abstractThe dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of CH2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.
dc.description.versionArticle: Version of Record (VoR)
dc.identifier.urihttp://hdl.handle.net/2097/39584
dc.language.isoen_US
dc.relation.urihttps://doi.org/10.1103/PhysRevA.96.043415
dc.rightsThis Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s).
dc.rights.urihttps://journals.aps.org/authors/transfer-of-copyright-agreement
dc.rights.urihttps://rightsstatements.org/page/InC/1.0/?language=en
dc.subjectOptical pumping
dc.subjectPhotodissociation
dc.subjectUltrafast phenomena
dc.titleCoulomb-explosion imaging of concurrent ${\mathbf{CH}}_{2}\mathbf{BrI}$ photodissociation dynamics
dc.typeText

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