Real-time observation of X-ray-induced intramolecular and interatomic electronic decay in CH2I2
Fukuzawa, Hironobu; Takanashi, Tsukasa; Kukk, Edwin; Motomura, Koji; Wada, Shin-ichi; Nagaya, Kiyonobu; Ito, Yuta; Nishiyama, Toshiyuki; Nicolas, Christophe; Kumagai, Yoshiaki; Iablonskyi, Denys; Mondal, Subhendu; Tachibana, Tetsuya; You, Daehyun; Yamada, Syuhei; Sakakibara, Yuta; Asa, Kazuki; Sato, Yuhiro; Sakai, Tsukasa; Matsunami, Kenji; Umemoto, Takayuki; Kariyazono, Kango; Kajimoto, Shinji; Sotome, Hikaru; Johnsson, Per; Schöffler, Markus S.; Kastirke, Gregor; Kooser, Kuno; Liu, Xiao-Jing; Asavei, Theodor; Neagu, Liviu; Molodtsov, Serguei; Ochiai, Kohei; Kanno, Manabu; Yamazaki, Kaoru; Owada, Shigeki; Ogawa, Kanade; Katayama, Tetsuo; Togashi, Tadashi; Tono, Kensuke; Yabashi, Makina; Ghosh, Aryya; Gokhberg, Kirill; Cederbaum, Lorenz S.; Kuleff, Alexander I.; Fukumura, Hiroshi; Kishimoto, Naoki; Rudenko, Artem; Miron, Catalin; Kono, Hirohiko; Ueda, Kiyoshi
Understanding strong X-ray induced phenomena is important for applications of X-ray free-electron laser imaging. Here, the authors show time-resolved measurements of X-ray free-electron laser induced electronic decay of CH2I2 molecule probed with NIR pulses and identify mechanisms behind different transient states lifetimes.
Keywords: Atomic and molecular interactions with photons; Chemical physics; Free-electron lasers
Journal:
Nature Communications, Volume:
10, Issue:
1, Starting Page:
2186,
Date:
2019
Rights:
CC-BY-NC-ND 4.0 license https://creativecommons.org/licenses/by-nc-nd/4.0/
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