Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy

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dc.contributor.author Wang, Xu
dc.contributor.author Le, Anh-Thu
dc.contributor.author Zhou, Zhaoyan
dc.contributor.author Wei, Hui
dc.contributor.author Lin, C. D.
dc.date.accessioned 2020-06-17T23:55:08Z
dc.date.available 2020-06-17T23:55:08Z
dc.date.issued 2017-08-28
dc.identifier.uri https://hdl.handle.net/2097/40723
dc.description.abstract We provide a unified theoretical framework for recently emerging experiments that retrieve fixed-in-space molecular information through time-domain rotational coherence spectroscopy. Unlike a previous approach by Makhija et al. (V. Makhija et al., arXiv:1611.06476), our method can be applied to the retrieval of both real-valued (e.g., ionization yield) and complex-valued (e.g., induced dipole moment) molecular response information. It is also a direct retrieval method without using iterations. We also demonstrate that experimental parameters, such as the fluence of the aligning laser pulse and the rotational temperature of the molecular ensemble, can be quite accurately determined using a statistical method.
dc.relation.uri https://doi.org/10.1103/PhysRevA.96.023424
dc.rights This Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s).
dc.rights.uri https://rightsstatements.org/page/InC/1.0/?language=en
dc.rights.uri https://journals.aps.org/authors/transfer-of-copyright-agreement
dc.subject High-order harmonic generation
dc.subject Multiphoton or tunneling ionization & excitation
dc.subject Molecules
dc.subject Schroedinger equation
dc.title Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy
dc.type Text
dc.date.published 2017
dc.citation.doi 10.1103/PhysRevA.96.023424
dc.citation.epage 023424-11
dc.citation.issn 2469-9934
dc.citation.issue 2
dc.citation.jtitle Physical Review A
dc.citation.spage 023424-1
dc.citation.volume 96
dc.description.version Article: Version of Record (VoR)


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This Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s). Except where otherwise noted, the use of this item is bound by the following: This Item is protected by copyright and/or related rights. You are free to use this Item in any way that is permitted by the copyright and related rights legislation that applies to your use. For other uses you need to obtain permission from the rights-holder(s).

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