Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy

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dc.contributor.author Wang, Xu
dc.contributor.author Le, Anh-Thu
dc.contributor.author Zhou, Zhaoyan
dc.contributor.author Wei, Hui
dc.contributor.author Lin, C. D.
dc.date.accessioned 2019-04-18T13:51:21Z
dc.date.available 2019-04-18T13:51:21Z
dc.date.issued 2017-08-28
dc.identifier.uri http://hdl.handle.net/2097/39577
dc.description Citation: Wang, X., Le, A.-T., Zhou, Z., Wei, H., & Lin, C. D. (2017). Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy. Physical Review A, 96(2), 023424. https://doi.org/10.1103/PhysRevA.96.023424
dc.description.abstract We provide a unified theoretical framework for recently emerging experiments that retrieve fixed-in-space molecular information through time-domain rotational coherence spectroscopy. Unlike a previous approach by Makhija et al. (V. Makhija et al., arXiv:1611.06476), our method can be applied to the retrieval of both real-valued (e.g., ionization yield) and complex-valued (e.g., induced dipole moment) molecular response information. It is also a direct retrieval method without using iterations. We also demonstrate that experimental parameters, such as the fluence of the aligning laser pulse and the rotational temperature of the molecular ensemble, can be quite accurately determined using a statistical method.
dc.language.iso en_US
dc.relation.uri 10.1103/PhysRevA.96.023424
dc.rights ©2017 American Physical Society
dc.rights.uri https://journals.aps.org/authors/transfer-of-copyright-agreement
dc.rights.uri https://rightsstatements.org/page/InC/1.0/?language=en
dc.subject High-order harmonic generation
dc.subject Multiphoton or tunneling ionization & excitation
dc.subject Molecules
dc.subject Schroedinger equation
dc.title Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy
dc.type Text
dc.date.published 2017
dc.citation.doi https://doi.org/10.1103/PhysRevA.96.023424
dc.citation.issn 1476-4688
dc.citation.issue 2
dc.citation.jtitle Physical Review A
dc.citation.spage 23424
dc.citation.volume 96
dc.citation Wang, X., Le, A.-T., Zhou, Z., Wei, H., & Lin, C. D. (2017). Theory of retrieving orientation-resolved molecular information using time-domain rotational coherence spectroscopy. Physical Review A, 96(2), 023424. https://doi.org/10.1103/PhysRevA.96.023424
dc.description.version Article: Version of Record (VoR)


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