Self-assembly at a nonequilibrium critical point
Date
2014-04-17
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Abstract
We use analytic theory and computer simulation to study patterns formed during the growth of two-component assemblies in two and three dimensions. We show that these patterns undergo a nonequilibrium phase transition, at a particular growth rate, between mixed and demixed arrangements of component types. This finding suggests that principles of nonequilibrium statistical mechanics can be used to predict the outcome of multicomponent self-assembly, and suggests an experimental route to the self-assembly of multicomponent structures of a qualitatively defined nature.
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Keywords
Two-component assemblies, Multicomponent self-assembly, Self-assembly, Nonequilibrium